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Fiddly to get to and you have to book in advance but if you can swing it bsky.app/profile/goat...

Map or no map, you are guaranteed to get lost there. Architecture, not necessarily brutalist: Just walk around Ginza and Omotesando to see wacky stuff. And Daikanyama T-Site is a pretty massive and remarkable bookstore

The Meguro Sky Garden is relatively obscure and a fun contrast.

Go out to the suburbs to see the Japanese equivalent of commie blocks: Danchi (団地)

A bit heavy to carry around?